Atomic Processes in Emission Characteristics of a Lithium Plasma Plume Formed by Double-Pulse Laser Ablation

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摘要 Highresolutionspectralanalysisoflithiumplasmaformedbysingleanddoublelaserablationhasbeenundertakentounderstandtheplume-laserinteraction,especiallyattheearlystagesoftheplasmaplume.Inordertoidentifydifferentatomicprocessesinevolvingplasma,timeresolvedspectralemissionstudiesatdifferentinter-pulsedelayshavebeenperformedforionicandneutrallithiumlinesemittingfromdifferentlevels.Alongwiththeenhancementinemissionintensity,alargelinebroadeningandspectralshift,especiallyinthecaseofexcitedstatetransitionLiI610.3nmhavebeenobservedinthepresenceofthesecondpulse.Thisbroadeningandshiftgraduallydecreasewithincreasingtimedelay.Anotherinterestingfeatureistheappearanceofamulti-componentstructureintheioniclineat548.4nmandthesecomponentschangeconverselyintoasinglestructureatthelaterstagesoftheplasma.Themulti-componentstructuresarecorrelatedwiththepresenceofdifferentvelocity(temperature)distributionsinnon-LTEconditions.AtomicanalysesbycomputingphotonemissivitycoefficientswithanADAScodehavebeenusedtoidentifytheaboveprocesses.
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出版日期 2013年03月13日(中国期刊网平台首次上网日期,不代表论文的发表时间)
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